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Highly sensitive and selective detection of ppb-level acetone sensor using WO3/Au/SnO2 ternary composite gas sensor

Zhu, Xiaojie; Ola, Oluwafunmilola; Li, Cong; Gao, Weixiang; Wang, Zhipeng; Dai, Changqian; Jiang, Yingchang; Sun, Shibin; Chang, Xueting

Authors

Xiaojie Zhu

Cong Li

Weixiang Gao

Zhipeng Wang

Changqian Dai

Yingchang Jiang

Shibin Sun

Xueting Chang



Abstract

Developing acetone sensors with high sensitivity and selectivity at ppb level is critical for medical diagnostics and environmental monitoring while facing serious challenges. In this work, we presented a ppb-level acetone sensor based on a WO3/Au/SnO2 ternary composite film with a sandwich structure that was obtained by combined methods of radio-frequency (RF) magnetron sputtering and ion beam sputtering. The structural and compositional characteristics of the WO3/Au/SnO2 composite film were analyzed by electron microscopy and X-ray photoelectron spectroscopy. The WO3/Au/SnO2 composite sensor possessed high response (28.9–50 ppm), low optimum working temperature (200 °C), fast response/recovery time (5.5/10.5 s), ultralow detection limit (170 ppb), good repeatability, and ideal long-term stability. The excellent gas-sensing performance of WO3/Au/SnO2 composite sensor could be mainly attributed to the construction of the heterostructures between different components and the chemical sensitization effect of the noble metal Au interlayer.

Citation

Zhu, X., Ola, O., Li, C., Gao, W., Wang, Z., Dai, C., Jiang, Y., Sun, S., & Chang, X. (2025). Highly sensitive and selective detection of ppb-level acetone sensor using WO3/Au/SnO2 ternary composite gas sensor. Ceramics International, 51(15), 20094-20102. https://doi.org/10.1016/j.ceramint.2025.02.173

Journal Article Type Article
Acceptance Date Feb 12, 2025
Online Publication Date Feb 13, 2025
Publication Date 2025-06
Deposit Date Feb 14, 2025
Publicly Available Date Feb 14, 2026
Journal Ceramics International
Print ISSN 0272-8842
Electronic ISSN 1873-3956
Publisher Elsevier
Peer Reviewed Peer Reviewed
Volume 51
Issue 15
Pages 20094-20102
DOI https://doi.org/10.1016/j.ceramint.2025.02.173
Keywords WO3/Au/SnO2 composite, Acetone sensor, Sputtering, Ppb-level, Heterostructures
Public URL https://nottingham-repository.worktribe.com/output/45314532
Publisher URL https://www.sciencedirect.com/science/article/pii/S0272884225008417