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Measuring radon-222 in soil gas with high spatial and temporal resolution

Huxtable, Darren; Read, David; Shaw, George

Authors

Darren Huxtable

David Read

George Shaw



Abstract

In order to exploit 222Rn as a naturally-occurring tracer in soils we need to sample and measure radon isotopes in soil gas with high spatial and temporal resolution, without disturbing in situ activity concentrations and fluxes. Minimization of sample volume is key to improving the resolution with which soil gas can be sampled; an analytical method is then needed which can measure radon with appropriate detection limits and precision for soil gas tracer studies. We have designed a soil gas probe with minimal internal dead volume to allow us to sample soil gas volumes of 45 cm3. Radon-222 is extracted from these samples into a mineral oil-based scintillation cocktail before counting on a conventional liquid scintillation counter. A detection limit of 320 Bq m-3 (in soil gas) is achievable with a one hour count. This could be further reduced but, in practice, is sufficient for our purpose since 222Rn in soil gas typically ranges from 2,000 - 50,000 Bq m-3. The method is simple and provides several advantages over commonly used field-portable instruments, including smaller sample volumes, speed of deployment and reliability under field conditions. The major limitation is the need to count samples in a liquid scintillation counter within 2 – 3 days of collection, due to the short (3.824 day) radioactive half-life of 222Rn. The method is not applicable to the very short-lived (55 second half-life) 220Rn.

Citation

Huxtable, D., Read, D., & Shaw, G. (2017). Measuring radon-222 in soil gas with high spatial and temporal resolution. Journal of Environmental Radioactivity, 167, https://doi.org/10.1016/j.jenvrad.2016.11.003

Journal Article Type Article
Acceptance Date Nov 1, 2016
Online Publication Date Nov 11, 2016
Publication Date Feb 1, 2017
Deposit Date Nov 7, 2016
Publicly Available Date Nov 11, 2016
Journal Journal of Environmental Radioactivity
Print ISSN 0265-931X
Electronic ISSN 1879-1700
Publisher Elsevier
Peer Reviewed Peer Reviewed
Volume 167
DOI https://doi.org/10.1016/j.jenvrad.2016.11.003
Keywords radon-222; 222Rn; soil gas; tube sampler; liquid scintillation counting; ionisation chamber
Public URL http://eprints.nottingham.ac.uk/id/eprint/38559
Publisher URL http://www.sciencedirect.com/science/article/pii/S0265931X16305434
Copyright Statement Copyright information regarding this work can be found at the following address: http://creativecommons.org/licenses/by-nc-nd/4.0

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Radon Manuscript Accepted 01Nov16.pdf (546 Kb)
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Copyright Statement
Copyright information regarding this work can be found at the following address: http://creativecommons.org/licenses/by-nc-nd/4.0





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