Analysis of contact area in a continuous application-and-peel test method for prepreg tack

Choong, G.Y.H.; Endruweit, A.; De Focatiis, D.S.A.

Abstract

The relationship between prepreg tack and the degree of intimate contact (DoIC) between prepreg and a rigid substrate was explored in the context of a continuous application-and-peel test method. Tack for a unidirectional prepreg tape was characterised for different surface combinations and varying test parameters (material feed rate, temperature) at a constant compaction pressure. Application of the prepreg to a transparent rigid substrate (glass), was carried out at matching test conditions to the prepreg tack measurements. Optical microscopy was utilised to acquire images of the contact area at the prepreg-glass interface. Image analysis of the micrographs enabled quantification of the contact area. The time- and temperature-dependent viscoelastic behaviour of the resin was explored directly on the prepreg using oscillatory parallel plate rheometry, and time-temperature superposition was applied to construct both tack and DoIC master curves. The shifted DoIC data showed that true contact area increases with decreasing shifted feed rates, until maximum contact area is achieved. Similarly, tack increases with decreasing shifted feed rates. However, at a critical feed rate, the bond failure mechanism switches from adhesive to cohesive failure. In cohesive failure, tack decreases with decreasing feed rate despite the high levels of DoIC.

• Journal Article Type: Article
• Acceptance Date: Mar 5, 2021
• Online Publication Date: Mar 11, 2021
• Publication Date: 2021-06
• Deposit Date: Mar 23, 2021
• Publicly Available Date: Mar 12, 2022
• Journal: International Journal of Adhesion and Adhesives
• Print ISSN: 0143-7496
• Publisher: Elsevier
• Peer Reviewed: Peer Reviewed
• Volume: 107
• Article Number: 102849
• DOI: https://doi.org/10.1016/j.ijadhadh.2021.102849
• Keywords: Tack; Epoxides; Peel; Prepreg
• Public URL: https://nottingham-repository.worktribe.com/output/5411230
• Publisher URL: https://www.sciencedirect.com/science/article/abs/pii/S0143749621000476