Anomalous Low Thermal Conductivity of Atomically Thin InSe Probed by Scanning Thermal Microscopy

Buckley, David; Kudrynskyi, Zakhar R.; Balakrishnan, Nilanthy; Vincent, Tom; Mazumder, Debarati; Castanon, Eli; Kovalyuk, Zakhar D; Kolosov, Oleg; Kazakova, Olga; Tzalenchuk, Alexander; Patan�, Amalia

Abstract

The ability of a material to conduct heat influences many physical phenomena, ranging from thermal management in nanoscale devices to thermoelectrics. Van der Waals two dimensional (2D) materials offer a versatile platform to tailor heat transfer due to their high surface-to-volume ratio and mechanical flexibility. Here, the nanoscale thermal properties of 2D indium selenide (InSe) are studied by scanning thermal microscopy. The high electrical conductivity, broad-band optical absorption and mechanical flexibility of 2D InSe are accompanied by an anomalous low thermal conductivity (). This can be smaller than that of low- dielectrics, such as silicon oxide, and it decreases with reducing the lateral size and/or thickness of InSe. The thermal response is probed in free-standing InSe layers as well as layers supported by a substrate, revealing the role of interfacial thermal resistance, phonon scattering, and strain. These thermal properties are critical for future emerging technologies, such as field effect transistors that require efficient heat dissipation or thermoelectric energy conversion with low-, high electron mobility 2D materials, such as InSe.

Citation

Buckley, D., Kudrynskyi, Z. R., Balakrishnan, N., Vincent, T., Mazumder, D., Castanon, E., …Patanè, A. (2021). Anomalous Low Thermal Conductivity of Atomically Thin InSe Probed by Scanning Thermal Microscopy. Advanced Functional Materials, 31(11), Article 2008967. https://doi.org/10.1002/adfm.202008967

• Journal Article Type: Article
• Acceptance Date: Dec 2, 2020
• Online Publication Date: Jan 12, 2021
• Publication Date: Mar 10, 2021
• Deposit Date: Dec 2, 2020
• Publicly Available Date: Jan 13, 2022
• Journal: Advanced Functional Materials
• Print ISSN: 1616-301X
• Electronic ISSN: 1616-3028
• Publisher: Wiley
• Peer Reviewed: Peer Reviewed
• Volume: 31
• Issue: 11
• Article Number: 2008967
• DOI: https://doi.org/10.1002/adfm.202008967
• Keywords: InSe; 2D semiconductors; scanning thermal microscopy; thermal conductivity; phonons
• Public URL: https://nottingham-repository.worktribe.com/output/5096691
• Publisher URL: https://onlinelibrary.wiley.com/doi/abs/10.1002/adfm.202008967?af=R
• Additional Information: This is the peer reviewed version of the following article: Buckley, D., Kudrynskyi, Z. R., Balakrishnan, N., Vincent, T., Mazumder, D., Castanon, E., Kovalyuk, Z. D., Kolosov, O., Kazakova, O., Tzalenchuk, A., Patanè, A., Anomalous Low Thermal Conductivity of Atomically Thin InSe Probed by Scanning Thermal Microscopy. Adv. Funct. Mater. 2021, 2008967, which has been published in final form at https://doi.org/10.1002/adfm.202008967. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions.