SANLIANG LING SANLIANG.LING@NOTTINGHAM.AC.UK
Associate Professor
© The Royal Society of Chemistry 2016. The metal-organic framework (MOF) material UiO-66 has emerged as one of the most promising MOF materials due to its thermal and chemical stability and its potential for catalytic applications. Typically, as-synthesised UiO-66 has a relatively high concentration of missing linker defects. The presence of these defects has been correlated with catalytic activity but characterisation of defect structure has proved elusive. We refine a recent experimental determination of defect structure using static and dynamic first principles approaches, which reveals a dynamic and labile acid centre that could be tailored for functional applications in catalysis.
Journal Article Type | Article |
---|---|
Acceptance Date | Mar 22, 2016 |
Online Publication Date | Mar 22, 2016 |
Publication Date | Jul 1, 2016 |
Deposit Date | Nov 20, 2018 |
Publicly Available Date | Jan 21, 2019 |
Journal | Chemical Science |
Print ISSN | 2041-6520 |
Electronic ISSN | 2041-6539 |
Publisher | Royal Society of Chemistry |
Peer Reviewed | Peer Reviewed |
Volume | 7 |
Issue | 7 |
Pages | 4706-4712 |
DOI | https://doi.org/10.1039/c5sc04953a |
Public URL | https://nottingham-repository.worktribe.com/output/1287934 |
Publisher URL | https://pubs.rsc.org/en/Content/ArticleLanding/2016/SC/C5SC04953A#!divAbstract |
Additional Information | : This document is Similarity Check deposited; : Supplementary Information; : Sanliang Ling (ORCID); : The Royal Society of Chemistry has an exclusive publication licence for this journal; OPEN ACCESS: This article is freely available. This article is licensed under a Creative Commons Attribution 3.0 Unported Licence (CC BY 3.0); : Single-blind; : Received 23 December 2015; Accepted 22 March 2016; Accepted Manuscript published 22 March 2016; Advance Article published 20 April 2016; Version of Record published 21 June 2016 |
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